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An auxiliary entangled pure state can enable an otherwise forbidden deterministic bipartite LOCC transformation while being returned exactly and uncorrelated with the output. Nielsen's pure-state conversion theorem reduces this to the displayed majorization condition on sorted squared Schmidt coefficients. It does not follow from a scalar comparison of entanglement entropies: tensoring changes which products occupy the largest cumulative-weight sums. An exact returned catalyst can be reused; merely restoring its marginal while allowing correlations is a different resource task.^[ref]

Entanglement dilution uses local operations and classical communication to prepare partially entangled states from maximally entangled states, such as Bell pairs. For many identical bipartite pure targets, the asymptotic cost in Bell pairs per target, allowing a vanishing approximation error, is their entanglement entropy in bits. The quantum typical subspace of the target's Schmidt coefficients has almost all its weight and dimension at most $2^{m(S+\delta )}$. A maximally entangled state of this dimension can be converted to the normalized truncated target by Nielsen's pure-state conversion theorem. The resulting state approaches the full target as the retained weight tends to one. Average monotonicity of pure-state entanglement entropy and entropy continuity give the converse lower bound. This is the reverse asymptotic task to entanglement concentration.

For real vectors of equal length and equal sum, write $x\prec y$ when ${\sum }_{j=1}^k{x}_j^{\downarrow }\le {\sum }_{j=1}^k{y}_j^{\downarrow }$ for every proper initial segment; the downward arrow means decreasing rearrangement. Majorization compares how unevenly a fixed total is distributed. The uniform probability vector is majorized by every probability vector, while $(1,0,\dots ,0)$ majorizes every probability vector. The order controls exact pure-state entanglement conversion in Nielsen's pure-state conversion theorem.

The Schmidt rank of a bipartite pure state cannot increase under local operations, even in a nonzero selected branch. A coefficient matrix $C$ changes under a local product operator to $AC{B}^T$, whose rank is at most that of $C$. For deterministic exact conversions the same conclusion follows from Nielsen's pure-state conversion theorem: at the input rank $r$, the majorization inequality forces all output coefficients after $r$ to vanish.

Write a source and target in Schmidt decomposition with squared coefficients $(1-s,s)$ and $(1-t,t)$, where $0<s,t\le 1/2$. If $s\ge t$, Nielsen's pure-state conversion theorem allows deterministic conversion. If $s<t$, the Schmidt-tail entanglement monotone gives $p\le s/t$. Alice attains this bound with a local two-outcome measurement in quantum mechanics whose success Kraus operator is $K_s=\mathrm{diag}(\sqrt{s(1-t)/(t(1-s))},1)$ and whose failure operator is $K_f=\mathrm{diag}(\sqrt{1-s(1-t)/(t(1-s))},0)$. They obey $K_s^{†}{K}_s+K_f^{†}{K}_f=I$. The successful unnormalized state is $\sqrt{s/t}$ times the target, and failure leaves a product state. A classical message tells Bob which branch occurred. Known local changes of Schmidt bases allow the same protocol for arbitrary two-qubit pure states with these coefficients.

Yes, the conversion can be deterministic using local operations and classical communication. Put $s=\sin \theta$ and $c=\cos \theta$. The initial state's squared Schmidt coefficients are $(1/2,1/2)$, while the target's decreasingly ordered squared Schmidt coefficients are $(c^2,s^2)$. Since $0<\theta <\pi /4$, one has $1/2<c^2$ and both pairs sum to one. ThusThe direction of this majorization is the allowed one in Nielsen's pure-state conversion theorem: maximal entanglement can be reduced by deterministic LOCC.

Here is an explicit protocol, so no conversion theorem need be assumed. The sender first applies a Pauli Z gate to remove the initial Bell-state minus sign. Starting from $|{\Phi }^{+}⟩$, she performs a two-outcome local measurement with Kraus operatorsThey define a valid measurement because $M_0^{†}{M}_0+M_1^{†}{M}_1=I$. The two unnormalized states after measurement areEach outcome has probability $1/2$. For outcome zero, the normalized state is already $s|00⟩+c|11⟩$. For outcome one, both parties apply Pauli X gates, obtaining the same state. The sender communicates only which outcome occurred. Finally the receiver applies a Pauli X gate, giving $s|01⟩+c|10⟩$ in either branch. This is deterministic two-qubit entanglement dilution, with total success probability one; it does not rely on postselection.

Put $s={\sin }^2\alpha$ and $t={\sin }^2\beta$. Then $0<s<t<1/2$, and the ordered squared Schmidt coefficients of the source and target are $(1-s,s)$ and $(1-t,t)$.

Nielsen's pure-state conversion theorem states that a deterministic exact conversion between bipartite pure states by LOCC exists precisely when the source's vector of squared Schmidt coefficients is majorized by the target's vector, with zero padding if needed. In the convention $x\prec y$, majorization requires ${\sum }_{j=1}^k{x}_j^{\downarrow }\le {\sum }_{j=1}^k{y}_j^{\downarrow }$ for every $k$, and equality of total sums. Here the first inequality would require $1-s\le 1-t$, but $s<t$ gives the reverse strict inequality. Thus exact conversion with certainty is impossible.

Use the usual asymptotic convention: the output approaches the desired $m(n)$-copy pure target in trace distance, and any recorded failure probability tends to zero. Define the binary entropyThe entanglement entropies per source and target are $E_{\psi }=h_2(s)$ and $E_{\varphi }=h_2(t)$. The asymptotic pure-state entanglement conversion rate isBoth achievability and the upper bound matter here.

For entanglement concentration, expand $n$ sources in their correlated computational basis. Every pair of strings of Hamming weight $k$ has the same amplitude $(1-s{)}^{(n-k)/2}{s}^{k/2}$. Alice measures only this weight, without resolving the individual string. Bob's string has the same weight automatically. Conditional on $k$, the normalized state is maximally entangled on $D_k=\left(\genfrac{}{}{0ex}{}{n}{k}\right)$ correlated strings. Its outcome probability is $\left(\genfrac{}{}{0ex}{}{n}{k}\right)s^k(1-s{)}^{n-k}$, a binomial distribution. By the weak law of large numbers, $k/n\to s$ in probability; Stirling's formula then gives $n^{-1}{\log }_2{D}_k\to h_2(s)$. A uniform Schmidt vector on $D_k$ entries is majorized by a uniform vector on $2^{\lfloor {\log }_2{D}_k\rfloor }$ entries padded with zeros. Thus Nielsen's pure-state conversion theorem converts the conditional state into that many Bell pairs exactly. For any fixed $\delta >0$, one obtains at least $n(E_{\psi }-\delta )$ Bell pairs with probability tending to one.

For entanglement dilution, consider the Schmidt strings of $m$ targets with probabilities $q_x$. The quantum typical subspace retains strings satisfyingThe retained probability $Q_m$ tends to one by the weak law applied to the independent variables $-{\log }_2{q}_{x_j}$. The number of retained strings is at most $2^{m(E_{\varphi }+\delta )}$, because their probabilities sum to at most one. Normalize the target after truncation to those strings. Its squared overlap with the full target is $Q_m\to 1$. A uniform Schmidt vector of dimension $2^L$, with $L=\lceil m(E_{\varphi }+\delta )\rceil$, is majorized by the truncated target's Schmidt vector padded with zeros: the sum of its largest $k$ entries is at least $k/2^L$. Hence $L$ Bell pairs prepare the truncated target exactly by LOCC. Its trace distance from the true target is $\sqrt{1-Q_m}\to 0$. Combining concentration and dilution achieves any rate $R<E_{\psi }/E_{\varphi }$. Choosing margins tending sufficiently slowly to zero attains the ratio as a limiting rate.

For the converse, average monotonicity of pure-state entanglement entropy follows from Concavity of Von Neumann entropy: a measurement by one party leaves the other party's reduction unchanged on average, so its average conditional entropy cannot increase. Refine local measurement records, including local discarded systems, to obtain pure output branches $\{p_r,|{\chi }_r⟩\}$ on the $m$ output qubits of each party. Iterating the concavity argument givesLet $|{\Phi }_m⟩=|\varphi {⟩}^{\otimes m}$ and let the squared-overlap error of the average output ${\rho }_{\mathrm{out}}$ be $\epsilon =1-⟨{\Phi }_m|{\rho }_{\mathrm{out}}|{\Phi }_m⟩\to 0$. Define $d_r=\sqrt{1-|⟨{\Phi }_m|{\chi }_r⟩{|}^2}$, the pure-state trace distance. Concavity of the square root gives ${\sum }_r{p}_r{d}_r\le \sqrt{\epsilon }$. Partial trace cannot increase trace distance, so the reduced states are also within $d_r$. The continuity bound for quantum conditional entropy, with trivial conditioning and local dimension $2^m$, impliesConsequentlywhich excludes a limiting rate exceeding $E_{\psi }/E_{\varphi }$.

The vanishing-error convention is essential. If exact deterministic conversion were required for every finite block, majorization would also require the largest squared Schmidt coefficient to satisfy $(1-s{)}^n\le (1-t{)}^m$, henceThis can be strictly smaller than the entropy ratio: at $s=0.1,t=0.2$, the two bounds are approximately $0.4722$ and $0.6496$. Thus the boxed rate answers the standard asymptotic task, rather than imposing unmentioned exact zero-error conditions on every finite block.

Let $r$ be the input Schmidt rank, so ${\lambda }_j=0$ for $j>r$ and ${\sum }_{j=1}^r{\lambda }_j=1$. If $r=d$, the output rank is already at most $r$. Otherwise, Nielsen's pure-state conversion theorem and majorization at $k=r$ giveThus all output coefficients beyond $r$ vanish, provingThis is monotonicity of Schmidt rank under LOCC. It also holds separately in any nonzero postselected branch: represent the input amplitudes by a matrix $C$; a local branch maps it to $AC{B}^T$, whose rank cannot exceed the rank of $C$. The deterministic result requested here follows already from the majorization criterion.

Nielsen's pure-state conversion theorem gives the exact deterministic LOCC criterion. Let the Schmidt decompositions be $|\psi ⟩={\sum }_j\sqrt{{\lambda }_j}|a_j{b}_j⟩$ and $|\varphi ⟩={\sum }_j\sqrt{{\mu }_j}|a_j^{\prime }{b}_j^{\prime }⟩$. The vectors $\lambda ,\mu$ consist of squared Schmidt coefficients, equivalently the eigenvalues of either reduced density operator. Order each in decreasing order and pad with zeros to a common length $d$.

Then deterministic conversion is possible if and only ifThis is majorization, with the input vector majorized by the output vector. The direction matters: a maximally entangled state has a uniform vector, which is majorized by a product state's vector $(1,0,\dots )$, so entanglement can be discarded by LOCC. The criterion is for certain exact conversion, without catalysts or postselection on a successful branch.

Nielsen's pure-state conversion theorem concerns exact deterministic transformations of bipartite pure states by local operations and classical communication. Let $\lambda (\psi )$ be the decreasing vector of squared Schmidt coefficients, equivalently the eigenvalues of either party's reduced density matrix, padded with zeros when necessary. ThenThe majorization relation means ${\sum }_{j=1}^k{\lambda }_j(\psi )\le {\sum }_{j=1}^k{\lambda }_j(\chi )$ for every $k$, with equality for the total sum. The direction allows a maximally entangled state to become a product state, not the reverse. Local-unitary invariance of reduced-state spectra alone would require equality of all the weights; measurements and communicated outcomes permit this larger class of conversions. A comparison of entanglement entropies alone is not a sufficient test in higher dimension.^[ref]

For the supplied states, the weight vectors and cumulative sums areAt $k=2$, $0.8>0.75$, violating the required inequality. The desired conversion is impossible with certainty using LOCC alone. The reverse conversion also fails, already at $k=1$, so these states are incomparable under this deterministic ordering.

Taking a tensor product with the catalyst multiplies every original weight by each catalyst weight. Regrouping the two local systems on Alice's side and the two on Bob's side leaves a Schmidt decomposition across the Alice–Bob partition. After sorting, the resulting weight vectors areThe actual nonnegative Schmidt amplitudes are $\sqrt{x_j}$ and $\sqrt{y_j}$; the displayed numbers are their squares. The cumulative sums areEvery component obeys $X_k\le Y_k$, so $x\prec y$. HenceThe final catalyst is exactly its initial state and is uncorrelated with the desired output. It can therefore be returned and reused. This is entanglement catalysis; it is stronger than merely retaining the same catalyst marginal while leaving correlations with the output.^[ref]

For the maximally entangled two-level auxiliary state, the sorted input weights are $(0.2,0.2,0.2,0.2,0.05,0.05,0.05,0.05)$, while the output weights are $(0.25,0.25,0.125,0.125,0.125,0.125,0,0)$. Their first four sums are $0.8$ and $0.75$. This maximally entangled auxiliary state cannot catalyze the conversion while being returned unchanged.

Nevertheless, $(0.5,0.5)\prec (0.6,0.4)$, so it can first be converted deterministically into the nonmaximal catalyst. The desired conversion can then proceed, after which Alice and Bob can return $|\varphi ⟩$, rather than the borrowed maximally entangled state. Turning that returned pair alone back into a maximally entangled pair would increase its entanglement entropy and is forbidden by LOCC. No joint restoration procedure can both keep the exact desired $|{\psi }_2⟩$ and return the original maximally entangled auxiliary state deterministically: its composition with the preceding steps would contradict the failed four-weight inequality above.

A bipartite pure state is entangled when it is not a product state. Its Schmidt decomposition is $|\psi ⟩={\sum }_i\sqrt{{\lambda }_i}|i_A{i}_B⟩$, where ${\lambda }_i\ge 0$ and ${\sum }_i{\lambda }_i=1$. More than one nonzero coefficient means entanglement. The two reduced density matrices have the same nonzero spectrum, and their Von Neumann entropy $-{\sum }_i{\lambda }_i{\log }_2{\lambda }_i$ is the pure-state entanglement entropy. A maximally entangled pair of qubits has one bit of this entropy.

For mixed states, classical correlations are not sufficient: a separable quantum state is a convex mixture ${\sum }_j{p}_j{\rho }_A^{(j)}\otimes {\rho }_B^{(j)}$, and entanglement means that no such decomposition exists. A reduced entropy alone no longer measures mixed-state entanglement. An entanglement witness or a suitable separability criterion can detect it.

Local unitary transformations preserve the Schmidt spectrum. More general local operations and classical communication can discard entanglement but cannot freely create it from a separable input. Nielsen's pure-state conversion theorem gives the exact deterministic criterion: $|\psi ⟩\to |\varphi ⟩$ is possible precisely when ${\lambda }^{\psi }\prec {\lambda }^{\varphi }$. In decreasing order, every partial sum for the input is no larger than the corresponding output sum, with equal totals. The direction matters: a uniform spectrum can be converted to a concentrated one; a product state cannot deterministically become a Bell pair.

A probabilistic local filter can concentrate a partially entangled pair. For $|\psi ⟩=\sqrt{\lambda }|00⟩+\sqrt{1-\lambda }|11⟩$ with $1/2\le \lambda <1$, Alice's successful operator $F=\mathrm{diag}(\sqrt{(1-\lambda )/\lambda },1)$ produces equal amplitudes. The outcome is a Bell pair with probability $2(1-\lambda )$; a complementary operator supplies a complete measurement. Failure is heralded, so there is no deterministic creation of a more entangled pair. This illustrates entanglement concentration.

Many-copy entanglement distillation and entanglement dilution connect noisy or nonuniform resources with standard Bell pairs. Entanglement enables quantum teleportation and other protocols, but classical communication is still required; the no-communication theorem excludes message transmission merely by choosing a distant local measurement.

Use the thin singular value decomposition $a=Ud{V}^{†}$, with $U^{†}U=I_N$, $V$ unitary and $d=\mathrm{diag}(d_k)$ nonnegative. Expanding its entries givesThe columns of $U$ and of $V^{\ast }$ are orthonormal, establishing the Schmidt decomposition. Bob's basis uses the complex-conjugated columns of $V$. Omitting that conjugation would not reproduce the coefficient matrix. The squared Schmidt coefficients are the eigenvalues of $a^{†}a$; equivalently $d^2=V^{†}{a}^{†}aV$ and $d=U^{†}aV$. The two reduced density matrices are $a{a}^{†}$ and $(a^{†}a{)}^T$, which have the same nonzero eigenvalues.

The printed coefficient $0.41231$ slightly rounds a normalized state: each squared norm is $0.9999995361$. Normalize before calculating an entropy. For the two states, the resulting Gram matrices are approximatelyFor a trace-one two-dimensional Hermitian matrix with diagonal entry $u$ and off-diagonal entry $c$, its eigenvalues areSort them decreasingly and take square roots:The Von Neumann entropy is $S=-{\lambda }_0{\log }_2{\lambda }_0-{\lambda }_1{\log }_2{\lambda }_1$. $\Psi$ is more entangled: its Schmidt weights are closer to equal and its reduced-state entropy is larger. Neither state is a product state or maximally entangled on its two-dimensional support.

By Nielsen's pure-state conversion theorem, deterministic LOCC conversion requires the input vector of squared Schmidt coefficients to be majorized by the output vector. Here $0.699941<0.894238$ and both sums are one, so $\lambda (\Psi )\prec \lambda (\Phi )$. Therefore $\Psi \to \Phi$ is possible deterministically; $\Phi \to \Psi$ is not. Entanglement can be discarded by local operations but cannot increase deterministically for these pure inputs. Probabilistic concentration is a separate question and is allowed below.^[ref]

There is a dimensional qualification in the proposed measurement. Write $P=|0_A^{\prime }⟩⟨0_A^{\prime }|+|1_A^{\prime }⟩⟨1_A^{\prime }|$. The two supplied measurement operators obeyThus their effects form a POVM on the occupied support, where $P$ is the identity. Alice's full space is three-dimensional, so these two operators alone do not sum to $I_3$. A full-space completion is $M_3=|2_A^{\prime }⟩⟨2_A^{\prime }|$. It has zero probability on either input, so it changes none of the requested outcomes. Strictly, the POVM consists of the effects $E_r=M_r^{†}{M}_r$; the specified $M_r$ additionally fix a quantum instrument and therefore the conditional states.

In the appropriate Schmidt basis for either input, write $|\psi ⟩=\sqrt{{\lambda }_0}|00⟩+\sqrt{{\lambda }_1}|11⟩$. The two outcomes have probabilitiesand normalized conditional statesThese formulas give both outcomes for each state by substituting its row of the table. For example,The two inputs have different Schmidt bases; the primed measurement basis is adapted separately to the state, as the question specifies, not one common unexamined laboratory basis.

For the $M_1$ outcome to be a maximally entangled state, its two amplitudes must be equal. HenceThe requested numerical results areThus $\Psi$ has the larger success probability, consistent with its greater initial entanglement. The $M_2$ branch cannot be balanced in the allowed angle range for either nonmaximal input: it would require $\tan \theta =\sqrt{{\lambda }_0/{\lambda }_1}>1$.

The success probabilities belong to this particular binary Schmidt filter. They are not the optimum over every possible quantum instrument. The diagonal success operator $\mathrm{diag}(\sqrt{{\lambda }_1/{\lambda }_0},1)$ instead gives the standard single-copy entanglement concentration probability $2{\lambda }_1$. Postselection can increase entanglement in the retained branch, while the outcome-averaged entanglement cannot increase under LOCC.