To Ernest Lawrence for the cyclotron.
cyclotrons produce the better images, but they are expensive/you have to move to them and order a timeslot.
Lab-based just use some X-ray source from the lab, so it is much move convenient e.g. for a pharmaceutical company doing a bunch of images. The Wikipedia image shows such a self-contained lab system: en.wikipedia.org/wiki/File:Freezed_XRD.jpg