Second-harmonic generation doubles optical frequency, hence halves the vacuum wavelength. It requires a nonzero effective second-order nonlinear optical susceptibility for the selected fields, overlap in the nonlinear medium, and enough intensity and interaction length for a useful signal. Bulk electric-dipole second-order response vanishes in an inversion-symmetric medium. Low absorption at both frequencies and phase matching prevent generated amplitudes from being lost or canceling during propagation. Pulses additionally need suitable temporal overlap and bandwidth acceptance.
For the stated lossless amplitude equations, choose real , input and no second-harmonic seed. Perfect phase matching admitsThe second equation follows by substituting the first into . Its derivative then equals , verifying the other coupled equation. Equivalently, ; changing the sign of does not change the pump profile. The intensity convention in the question therefore givesTheir sum is , as follows directly from the supplied equal-coupling equations. This uses their normalization; physically normalized photon-flux equations can place frequency factors in the two coupling coefficients. A nonzero input harmonic would require a different boundary-value solution.
For an undepleted pump at nonzero mismatch, direct integration givesHere . The perfectly matched small-signal curve grows quadratically and its depleted continuation saturates. For , destructive phase accumulation reduces output; in the undepleted limit its endpoint is of the matched small-signal output. For , successive regions alternately generate and cancel harmonic amplitude, giving rapid low-amplitude oscillations with spatial period . For substantial depletion, the complete curve also depends on ; specifying mismatch alone does not determine a unique numerical sketch.
For the separated crystals, use the undepleted approximation and perfect matching inside each crystal. Up to a common output phase, the harmonic generated in the first crystal contributes , while the second crystal contributes . The different phases come from propagation of an already generated harmonic versus propagation of two pump factors through the gap. Ideal antireflection coatings remove the multiple-reflection complication. ThusThis is two-crystal second-harmonic interference. Maxima require . With nonzero dispersion, their spacing is , where is the pump vacuum wavelength. If the gap has no index difference between these frequencies, every separation is constructive within this ideal propagation model.
Finite depletion makes the amplitude entering the second crystal smaller and permits coherent backconversion, so the simple cosine-squared envelope no longer applies and the total converted intensity cannot exceed . The gap phase remains periodic. In the ideal identical lossless case the constructive setting is equivalent to a matched crystal of length , giving . The opposite relative phase can make the second crystal reverse the first conversion, restoring the pump and leaving zero harmonic. Thus depletion does not necessarily fill an ideal destructive minimum; unequal crystals, loss or other phase errors can spoil that cancellation.
