 Solution

For a normalized state $|\psi (t_F;f)⟩$ driven by the admissible control $f$, maximizeHere $A$ is the specified Hermitian operator, $t_F$ the final time, and the dependence on $f$ is through the Schrödinger equation. The objective is real and is exactly the desired expectation value, so increasing it increases the requested observable. A control-resource penalty may be included when the admissible set does not already constrain field strength or fluence.