 Third-order correlation brightness weighting

Third-order correlation brightness weighting is the way bright shots contribute disproportionately to an averaged nonlinear correlation trace. A normalized average trace is a weighted mean of shot-normalized shapes, with weights set by their central correlation signals rather than by how often the shots occur.

Let a nonnegative, background-corrected third-order trace on shot $j$ be $A_j(\tau )$. Define its central signal $B_j=A_j(0)>0$ and normalized shape $r_j(\tau )=A_j(\tau )/B_j$. Then the experimentally distinct averages areand the equal-shot mean $R_{\mathrm{shot}}(\tau )=N^{-1}{\sum }_j{r}_j(\tau )$. The nonnegative $w_j$ sum to one, but are equal only when the $B_j$ are equal. Here “central” denotes the specified zero-delay signal, not whichever noisy sample happens to be the largest.

For identical pulse shapes multiplied by intensity factors $K_j$, the ideal integral $A_j(\tau )=\int I_j^2(t)I_j(t+\tau )dt$ scales as $K_j^3$. The primary correlator implements this three-intensity-factor gate using second-harmonic generation followed by sum-frequency generation.^[ref] If shapes change, $B_j$ can depend on duration and overlap as well as brightness, so pulse energy alone need not determine the weight.

An original two-class example has equally frequent classes with $(B,r)=(1,0.01)$ and $(8,0.10)$ at one chosen delay. Their equal-shot mean ratio is $0.055$, but the normalized summed trace givesThe bright class supplies eight ninths of the central signal despite representing only half the shots. Neither result is an arithmetic mistake: they estimate different summaries of the stipulated ensemble.

For an ensemble with finite moments and $\mathbb{E}[B]>0$, the distinction can be expressed exactly through covariance:Unchanged normalized shape makes the covariance zero, even with large brightness fluctuations. Shape–brightness dependence can make it nonzero; cubic intensity-noise bias in pulse correlation alone does not prove a contrast change.

A shot-resolved pulse-contrast estimator needs synchronized intensity information and a stated selection rule. Thresholding weak shots or dividing by a noisy central signal can introduce further selection and ratio errors. Report whether normalization occurred before or after averaging, retain detector baseline subtraction, and test readout linearity. A smooth averaged trace is not a representative single shot unless those assumptions are justified.