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Physical Review Letters 83, 3566–3569. Original account of entanglement catalysis by Daniel Jonathan and Martin B. Plenio.

Author preprint: arxiv.org/abs/quant-ph/9905071

Nielsen's pure-state conversion theorem concerns exact deterministic transformations of bipartite pure states by local operations and classical communication. Let $\lambda (\psi )$ be the decreasing vector of squared Schmidt coefficients, equivalently the eigenvalues of either party's reduced density matrix, padded with zeros when necessary. ThenThe majorization relation means ${\sum }_{j=1}^k{\lambda }_j(\psi )\le {\sum }_{j=1}^k{\lambda }_j(\chi )$ for every $k$, with equality for the total sum. The direction allows a maximally entangled state to become a product state, not the reverse. Local-unitary invariance of reduced-state spectra alone would require equality of all the weights; measurements and communicated outcomes permit this larger class of conversions. A comparison of entanglement entropies alone is not a sufficient test in higher dimension.^[ref]

For the supplied states, the weight vectors and cumulative sums areAt $k=2$, $0.8>0.75$, violating the required inequality. The desired conversion is impossible with certainty using LOCC alone. The reverse conversion also fails, already at $k=1$, so these states are incomparable under this deterministic ordering.

Taking a tensor product with the catalyst multiplies every original weight by each catalyst weight. Regrouping the two local systems on Alice's side and the two on Bob's side leaves a Schmidt decomposition across the Alice–Bob partition. After sorting, the resulting weight vectors areThe actual nonnegative Schmidt amplitudes are $\sqrt{x_j}$ and $\sqrt{y_j}$; the displayed numbers are their squares. The cumulative sums areEvery component obeys $X_k\le Y_k$, so $x\prec y$. HenceThe final catalyst is exactly its initial state and is uncorrelated with the desired output. It can therefore be returned and reused. This is entanglement catalysis; it is stronger than merely retaining the same catalyst marginal while leaving correlations with the output.^[ref]

For the maximally entangled two-level auxiliary state, the sorted input weights are $(0.2,0.2,0.2,0.2,0.05,0.05,0.05,0.05)$, while the output weights are $(0.25,0.25,0.125,0.125,0.125,0.125,0,0)$. Their first four sums are $0.8$ and $0.75$. This maximally entangled auxiliary state cannot catalyze the conversion while being returned unchanged.

Nevertheless, $(0.5,0.5)\prec (0.6,0.4)$, so it can first be converted deterministically into the nonmaximal catalyst. The desired conversion can then proceed, after which Alice and Bob can return $|\varphi ⟩$, rather than the borrowed maximally entangled state. Turning that returned pair alone back into a maximally entangled pair would increase its entanglement entropy and is forbidden by LOCC. No joint restoration procedure can both keep the exact desired $|{\psi }_2⟩$ and return the original maximally entangled auxiliary state deterministically: its composition with the preceding steps would contradict the failed four-weight inequality above.