A density operator satisfies
An Hermitian matrix has real parameters, and the trace condition removes one, leaving
real free parameters.
If , equality of expectation values requires
Therefore
The spin commutators are
Set
Purity gives , so the supplied sign determines
For , choose the overall phase so that the upper component is nonnegative. The normalized state is
If , it is simply up to phase.
For a mixed spin-half state, the Bloch vector formula gives
Physical consistency is equivalent to the resulting Bloch vector having length at most one.
Three linearly independent Hermitian operators do not always suffice. The operators
are linearly independent, but the first expectation is always one and none detects the component. States with Bloch vectors and have identical expectations for all three. The correct criterion for informationally complete three-observable qubit tomography is that the three traceless parts span the Pauli space.

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