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The isomorphic pair is $A_8\cong PS{L}_4(2)$; $PS{L}_3(4)$ is different. All three have order $20160$, so order alone does not settle the question; explicitly $|PS{L}_3(4)|=(64-1)(64-4)(64-16)/(3\cdot 3)=20160$. We give a concrete realization and an element-order distinction.

On $W={\bigwedge }^2{\mathbb{F}}_2^4$, the Pfaffian isIt is a nonsingular plus-type quadratic form: the three displayed pairs give a hyperbolic decomposition. Change of basis multiplies the Pfaffian by the determinant, which is always one in $G{L}_4(2)$. Hence the exterior-square realization of PSL4 over F2 embeds $G{L}_4(2)$ into $O_6^{+}(2)$. The kernel of a group homomorphism is trivial: an element acting trivially on the exterior square fixes every decomposable two-space, then every one-space as an intersection of two-spaces, and hence is a scalar; over ${\mathbb{F}}_2$ this scalar is one.

For a second model let $E$ be the even-weight vector subspace of ${\mathbb{F}}_2^8$ and quotient by the all-one vector. The dot product descends to a nondegenerate alternating bilinear form on the six-dimensional quotient, andis well defined, since complementing an even subset changes half its weight from $w/2$ to $4-w/2$. It has $(1+70+1)/2=36$ zero vectors, so is plus type. Coordinate permutations give a faithful $S_8$ action: fixing the quotient fixes each weight-two subset, because its complement has weight six, and fixing all two-subsets forces the identity permutation.

From the independently derived symplectic order and quadratic orbit count below,Thus $O_6^{+}(2)\cong S_8$ and the image of $G{L}_4(2)=S{L}_4(2)=PS{L}_4(2)$ is its index-two subgroup $A_8$. The index-two subgroup is unique: a nontrivial group homomorphism $S_8\to C_2$ sends every transposition to the same nonidentity element and is the sign map.

To separate $PS{L}_3(4)$, observe that $A_8$ contains $(12345)(678)$ of order 15. An odd-order projective element of $PS{L}_3(4)$ lifts to a semisimple linear operator, since its order upstairs divides three times an odd order in characteristic two. The possible eigenspace degree patterns are $1+1+1$, $2+1$ and $3$. In the split case all eigenvalues have order dividing three, so the projective element has no order 15. In the $2+1$ case the eigenvalues are $\lambda ,{\lambda }^4,{\lambda }^{-5}$ with $\lambda \in {\mathbb{F}}_{16}^{\times }$; its fifth power is scalar because ${\lambda }^{15}=1$, so its projective order divides five. In the irreducible case the determinant-one torus has order $4^2+4+1=21$ and quotienting its scalar subgroup of order three gives projective order dividing seven. There is therefore no element of order 15 in $PS{L}_3(4)$.

Several small-parameter coincidences connect the finite classical groups to permutation groups. The projective-line action immediately gives $PS{L}_2(2)\cong S_3$, $PS{L}_2(3)\cong A_4$, $PG{L}_2(3)\cong S_4$ and $PS{L}_2(4)\cong A_5$ by faithful actions of degrees three, four and five and their orders. Also $PS{L}_2(5)\cong A_5$: its involutions have Klein-four centralizers, giving five Sylow subgroups; their conjugation action is faithful and embeds its order-60 simple group into $S_5$. Simplicity here can be checked from class sizes $1,15,20,12,12$: no proper nontrivial normal class union has order dividing 60. The same five-subgroup action extends to $PG{L}_2(5)$, with trivial kernel of a group homomorphism and order 120, giving $S_5$. Indeed its kernel intersects $PS{L}_2(5)$ trivially, so centralizes that normal subgroup. Commuting projectively with both upper and lower elementary unipotents forces a representing matrix to be scalar, so this kernel is trivial.

The less immediate coincidence $PS{L}_2(9)\cong A_6$ can be exhibited on the ten unordered triple partitions used in Question 4. Let $a=(123)$, $b=(456)$, $w=(12)(36)$, assign $\infty$ to $123\mid 456$ and $0$ to $126\mid 345$, and label the other partitions by applying $a^x{b}^y$ to the zero partition, with $t=x+iy\in {\mathbb{F}}_9$ and $i^2=-1$. Inspection of these nine partitions givesTranslations and inversion generate $PS{L}_2(9)$: conjugating the upper unitriangular matrices by inversion gives the lower ones, and elementary elimination generates $S{L}_2(9)$. Their projective action has order $9(9^2-1)/2=360$. These partition permutations come from even permutations of six letters, whose partition action is faithful as proved below; hence they fill $A_6$.

Finally, on the even-weight module of ${\mathbb{F}}_2^6$ modulo its all-one vector, coordinate permutations preserve a nondegenerate alternating bilinear form in dimension four and act faithfully, again by the weight-two-subset argument. Both $S_6$ and $S{p}_4(2)$ have order 720, proving $S{p}_4(2)\cong S_6$, with commutator subgroup $A_6$. These examples illustrate both the need to quotient group centers and the low-rank exceptions to general simplicity. They do not make equal orders sufficient for group isomorphism, as the two order-20160 examples already demonstrate.