 Optical prepulse

An optical prepulse is a secondary optical pulse arriving before the reference main pulse. The sign of its delay is part of the definition: choose the main pulse at $t=0$, so a prepulse has negative arrival time. A weak earlier pulse and an equally weak optical postpulse can affect a target differently when the material retains a response to the earlier illumination. Temporal order therefore carries information that one total laser pulse energy does not.

An original separated rectangular-profile example uses a main pulse of duration $100\mathrm{fs}$ and a prepulse of duration $10\mathrm{ps}$ centred $50\mathrm{ps}$ earlier. Let the prepulse's peak radiant power be $10^{-4}$ of the main peak. The optical pulse temporal contrast is $10^4$, but the energy ratio isThus the prepulse carries $1/101\approx 0.990\%$ of the two-pulse energy. If the main pulse carries $1\mathrm{mJ}$, the prepulse carries $10\mu \mathrm{J}$. These stipulated disjoint power profiles have no field-overlap term, and the main pulse's full width at half maximum does not reveal the earlier contribution.

A temporal diagnostic needs both sufficient delay coverage and calibrated dynamic range. The single-shot third-order correlator paper motivates its asymmetric response by contrasting it with the symmetric second-order trace, which loses the distinction between before and after.^[ref] Its delay axis still needs a known physical reference. A third-order pulse correlation ghost from a real postpulse can appear on the prepulse side; interpreting every small lobe as earlier light would be incorrect.

Repeating the measurement while varying an independently characterized optical delay helps assign temporal order. Record the detector baseline subtraction, coverage and response width along with the trace. A nondetection means a limit within those measurement conditions, rather than proof of zero early optical energy.