Attosecond pulse train 2026-10-18
An attosecond pulse train contains repeated short optical pulses. For a group of odd multiples of a common driving frequency, the separation is half the driving period when the relative spectral phases recur. The construction resembles mode locking, but the participating components come from high harmonic generation, rather than separate resonant modes of a laser oscillator.
A transform-limited pulse needs coherent phases across its contributing frequency range. A laser's usable gain bandwidth therefore sets a duration scale through the time-bandwidth product, as displayed. The wavelength interval must first be converted to frequency; the simple conversion is only a narrow-band approximation. Numerical constants depend on pulse shape and width convention: a Gaussian intensity envelope has . A hard gain interval is not automatically a spectral FWHM. Mode locking can arrange the longitudinal modes' phases, while group velocity dispersion must be controlled to approach the transform limit. The cavity round-trip time sets pulse spacing, rather than this bandwidth-limited width.
Mode locking 2026-10-18
Mode locking fixes relative phases between longitudinal normal modes of a laser, allowing short optical pulses. The same optical spectrum with wandering relative phases would not supply that stable pulse train.[ref]
Here is an original finite-mode model, with the convention that a positive frequency has time dependence :
These field coefficients follow a Gaussian function and have aligned phases at . Choose and write . Since for every integer ,
The pulse light intensity repeats every although the field needs four periods to repeat. At the pulse centers, , , and . A detector of light intensity alone therefore cannot distinguish this offset from zero. This model has far fewer teeth than a practical optical comb; its normalized time and frequency scales are chosen to make the carrier oscillations visible.
Figure 1.
Repeated pulse envelopes can conceal a changing carrier phase
. Original finite sum of 17 normal modes weighted using a Gaussian function, with . Both panels represent the same complex field: the upper panel shows its real part and magnitude; the lower panel shows its field-amplitude coefficients. This is a dimensionless model, not historical measurement data. Details.
A short proof of the converse uses the Fourier series. If , then is periodic with period . Its Fourier series has frequencies ; restoring the removed factor shifts every tooth by . A finite observation time broadens the spectral peaks; it does not change this ideal infinite-train relation.
Use mode locking to phase-lock many longitudinal cavity modes; their repeated constructive interference produces short optical pulses. A saturable absorber can select this pulsed operation. A fundamental repetition rate corresponds to a round trip, or an optical round-trip length ; a linear air-filled cavity would therefore be about long. A compact alternative is a faster mode-locked oscillator followed by pulse selection and, if required, amplification. Ordinary Q-switching alone generally does not provide pulses.[ref]
Mode locking fixes the relative phases of a laser's longitudinal cavity modes, so they interfere constructively in a regularly repeating short pulse rather than producing an uncontrolled temporal waveform. Active mode locking uses an externally driven modulation of loss, gain or phase at the cavity repetition frequency; an electro-optic modulator acting as a periodic transmission gate is one example. Passive mode locking uses the pulse itself to select a high-intensity waveform: a saturable absorber has lower loss at the pulse peak and can lock the phases without an external clock. A semiconductor saturable-absorber mirror is a practical example. Gain recovery, dispersion and saturation must support a stable circulating pulse.
Using the complex-field convention in the question, add the fields of all the oscillating modes. Set , so that . Then
There are terms with the printed inclusive indexing. The sum is periodic with period
which is the separation of adjacent pulses when many modes contribute. The carrier factor need not repeat over this interval.
To specify the carrier-envelope phase sign, write the real field near pulse , with , as . Its cosine phase is . Since ,
Equivalently, the phase in the complex convention advances by . This is the negative of the cosine phase, not a different physical prediction. The carrier-envelope offset frequency fixes this pulse-to-pulse slip. It matters for a few-cycle field's peak electric waveform and for locating an optical frequency comb's lines; a stable intensity envelope alone does not fix the slip.
Figure 1.
Identical pulse envelopes with changing carrier phase; the plotted phase labels use the complex-field convention
. Details.
If and , many closely spaced modes lie under the spectral Gaussian and the cutoffs have negligible weight. Near one pulse, replace the sum by its continuum integral:
The Fourier transform of a Gaussian therefore gives
This is a local single-pulse approximation. The discrete spectrum produces its periodic replicas; extending one Gaussian over all time would lose them. The temporal light intensity is proportional to , while the spectral intensity envelope is proportional to . Their full widths at half maximum are
In ordinary frequency this time-bandwidth product is . The spectral phases are flat, so this is a transform-limited pulse; chirp would generally increase its temporal width.
Q-switching stores excitation in a pumped laser gain medium while preventing oscillation, then rapidly changes the optical cavity from high loss, or low quality factor, to low loss, or high quality factor. The initially suppressed stimulated field can then grow rapidly from a seed and deplete a large population inversion in a short pulse. The resulting peak power is much higher than for continuous operation at the same average pumping rate. This is energy storage and release, rather than the phase locking of many longitudinal modes used in mode locking.
An active implementation uses a Pockels cell and a polarizer. An applied voltage makes the cell change the intracavity polarization, causing the polarizer to introduce sufficient loss to prevent lasing while pumping builds the inversion. Rapidly changing the voltage removes that loss and opens the high-Q state. The switching time should be short relative to the pulse build-up and depletion times. A saturable absorber provides an alternative passive Q switch: its absorption decreases as the intracavity intensity rises.
In mode locking, fixed relative phases between many longitudinal normal modes produce constructive interference during a short part of each optical resonator round trip. The round-trip time sets the repetition period. The available coherent gain bandwidth, the number of locked normal modes, the spectral phase, and residual group velocity dispersion determine the optical pulse duration.
For consecutive equally weighted normal modes of angular frequency spacing , their wave amplitude sum is proportional to
Its central peak has width of order , while its repetition period is . A transform-limited pulse therefore becomes shorter as more coherent gain bandwidth is used. This mechanism can give picosecond or femtosecond optical pulses: it does not require depletion of the whole stored population inversion during each peak, as Q-switching does. Mode locking generally accesses a much shorter time-bandwidth product scale than the gain-discharge time of Q-switching.
The gain bandwidth must be expressed as a frequency range:
The gain bandwidth limit on a laser pulse then gives
The numerical coefficient depends on the pulse shape and width definition. For example a Gaussian pulse whose intensity spectral FWHM actually filled this width would have a transform-limited intensity duration about . A hard gain interval does not by itself specify such a FWHM. Reaching the estimated scale requires coherent mode locking and control of group velocity dispersion; the cavity round-trip time determines the pulse separation. An intensity autocorrelation measurement can estimate the pulse duration once its shape is specified.