Only the two-qubit experiment is possible. Choose the spin singlet state
It has eigenvalue under each of , and . Thus measuring either qubit in the same Pauli basis as the other always gives opposite eigenvalue labels. Each opposite-label pair occurs with probability . More generally, collective-unitary covariance of the two-qubit singlet ensures opposite outcomes in any common orthonormal qubit basis.
For the sequential experiment, the first outcome is uniformly distributed and the Lüders rule prepares the corresponding eigenstate. Certain opposite outcomes in the computational basis force the fixed unitary matrix to have the form
Certain opposite Hadamard basis outcomes require , hence . Therefore . But this operator preserves the two Pauli Y eigenstate rays: it gives the same Y-basis label on the second measurement, rather than the opposite one. This contradicts the third set of observations.
Equivalently, flipping all three bases would require , , and . Conjugating in these two ways gives both and , an impossibility. This three-axis obstruction to unitary qubit orthogonalization is a finite test of the obstruction behind the universal NOT gate.
Figure 1.
Sequential qubit correlations and singlet correlations differ in the third basis
. Original exact predictions, not measured data. With a maximally mixed initial qubit, the sequential experiment using U=Y has opposite Z and X results but equal Y results. A singlet pair has opposite results in all three bases. Correlation +1 means equal labels and −1 means opposite labels. Details.

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