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Walther Bothe and Herbert Becker observed penetrating radiation from beryllium struck by alpha particles before James Chadwick's interpretation.^[ref]

Irène Joliot-Curie and Frédéric Joliot found that adding material containing hydrogen increased ionization, interpreting the ejected protons as Compton scattering recoils from extremely energetic gamma rays. James Chadwick tested this interpretation against nuclear recoils in other elements.^[ref]

The counter coupled a small ionization chamber to an amplifier and oscillograph: charged particles produced ions, and the electrical signal gave a deflection. With Norman Feather, James Chadwick also observed nitrogen recoil tracks in a cloud chamber.^[ref]

The apparatus used polonium on silver facing beryllium inside an evacuable vessel. Paraffin wax before the aluminium counter window supplied recoil protons; intervening aluminium screens measured their particle range. Deflections were photographed on bromide paper. The first counter contained air; later fillings included hydrogen, helium, nitrogen, oxygen and argon. Counts with wax absent included gas recoils; wax insertion added entering protons. Thick lead between source and counter hardly changed the initial counts, testing penetration against the low background.^[ref]

The diagram separates two routes to a signal: a proton entering from the wax and a nuclear recoil created inside the chamber gas. Its lower row is a logical summary, rather than a reconstructed experimental trace. In either route the observed ionization belongs to a charged secondary particle; identifying the incident radiation requires an additional collision model.

In the February letter, a photon interpretation requiring about $52\mathrm{MeV}$ for the protons predicted only about $0.4\mathrm{MeV}$ for nitrogen recoils, below the observed ionization. Here $1\mathrm{MeV}=10^6$ electronvolts. James Chadwick proposed a neutral particle near the proton mass and the nuclear reactionThese are the letter's approximate historical values, not a modern mass determination.^[ref]

Why compare two materials? A gamma ray is a photon, so its incident momentum is $E_{\gamma }/c$, where $c$ is the speed of light. A slow massive projectile instead has momentum $mv$ and kinetic energy $m{v}^2/2$. The relationship between incoming momentum and energy therefore changes. An elastic collision model must explain the recoil endpoints for both target masses with the same incident projectile population. Calling the radiation neutral supplies no such agreement by itself.

The original measurements depended on particle range calibration, material in the path, detector response and whether a recoil was fully stopped in the sensitive gas. Large deflections alone need not specify a complete recoil energy. The calculations below expose the ideal collision assumptions behind the inference; applying them to a measured spectrum requires checking those assumptions.

A single recoil endpoint leaves a tradeoff between incident speed and projectile mass. Two targets can remove the unknown incident speed. Assume both runs sample the same maximum projectile speed $v$ and that single elastic collisions reach the endpoint. For initially stationary target masses $M_1<M_2$, let their maximum recoil speeds be $u_1,u_2$. The maximum elastic recoil energy fraction calculation givesIf energies rather than speeds are inferred, use $R=\sqrt{T_{1,\max }{M}_2/(T_{2,\max }{M}_1)}$. The energy ratio itself is not the speed ratio.

For the stipulated $4\mathrm{MeV}$ example, hydrogen and nitrogen giveThe inferred mass then determines $v=u_1(m+M_1)/(2m)$. Changing the assumed mass to improve one recoil endpoint changes the prediction for the other: this is the constraining power of the comparison.

James Chadwick's June paper instead used approximate endpoints $u_p=3.3\times 10^{7}m/s$ and $u_N=4.7\times 10^{6}m/s$, obtaining $m/m_p\simeq 1.15$; it allowed roughly ten percent uncertainty in $u_N$. This was a rough mass comparison.^[ref]

The inverse calculation has useful built-in checks. A positive finite mass requires $1<R<M_2/M_1$. As $R$ approaches $1$, distinguishing large projectile masses becomes difficult. Differentiation givesUncertain recoil endpoints therefore produce an uncertain inferred mass; the collision model cannot turn imprecise range measurements into exact spectroscopy. If different target runs select different incident energy groups, the common-$v$ cancellation also fails.

For comparison, Compton scattering of a photon of energy $E_{\gamma }$ from a stationary free target of mass $M$ has the exact relativistic endpointThis follows by combining momentum conservation with the target's relativistic energy, maximizing transfer when the photon reverses direction. Unlike the massive-projectile calculation, this equation does not approximate the incident photon as a nonrelativistic particle.

As a separate, explicitly hypothetical test, take $m_p{c}^2=938\mathrm{MeV}$ and target rest energies $938\mathrm{MeV}$ and $14\times 938\mathrm{MeV}$. To reproduce the stipulated hydrogen recoil endpoint $T=4\mathrm{MeV}$, the photon would need $E_{\gamma }\simeq 45.36\mathrm{MeV}$. The same photon would give the heavier target at most $0.311\mathrm{MeV}$, whereas the stipulated massive projectile gave $0.996\mathrm{MeV}$. This is the structure of a two-target discrimination, not a transcription of a 1932 measurement. Actual radiation can contain more than one energy group or both photons and neutrons; a useful model must account for the observed endpoints and their origin together.