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A physicist who researches high harmonic generation and ultrafast Electron dynamics.^[ref]

Attosecond physics resolves changes on the scale of $10^{-18}$ seconds, especially Electron dynamics. Its central trick is to convert a short optical event into an experimentally accessible energy or phase change. A broad optical spectrum provides the ingredients for a short optical pulse; their spectral phases determine when those ingredients add constructively. High harmonic generation supplies the optical spectrum, while RABBITT and attosecond streaking supply complementary timing measurements. XUV denotes extreme ultraviolet radiation.

There are two separate timing problems: characterize the incident optical pulse, then infer the response of the target. A photoelectron measurement mixes the incident spectral phase, the target's transition response and the probing electric field. Recovering one requires constraints on the others. These methods measure distributions of photoelectron energies over repeated shots, rather than photographing a moving atomic orbital.

An attosecond pulse train contains repeated short optical pulses. For a group of odd multiples of a common driving frequency, the separation is half the driving period when the relative spectral phases recur. The construction resembles mode locking, but the participating components come from high harmonic generation, rather than separate resonant modes of a laser oscillator.

High harmonic generation converts an intense driving electric field into radiation at high integer multiples of its frequency. High harmonic generation in a gas is a process in nonlinear optics: an Electron can leave a neutral target by tunnel ionization, gain kinetic energy in the driving electric field, and return to radiate upon recombination. This three-step picture is an approximate account of a probability amplitude for emission in quantum mechanics, not a measured path of one Electron.^[ref]

Why odd multiples? In an ideal centrosymmetric gas driven by a single frequency, assume the radiating electric dipole moment satisfies $d(t+T/2)=-d(t)$, where $T$ is the driving period. Its Fourier series coefficient obeys $d_q=-(-1{)}^q{d}_q$, so every even coefficient vanishes. A finite envelope, an oriented target or an additional driving frequency can invalidate that symmetry argument. Producing many odd components also does not prove that their spectral phases form a short optical pulse.

The 1988 report involving Anne L'Huillier observed odd multiples of a $1064\mathrm{nm}$ driving wavelength in rare gases, reaching order 33 in argon. The unexpectedly slow fall of yield beyond the fifth order supplied a broad spectral plateau. A spectral observation alone did not establish the relative spectral phases needed for an attosecond pulse train.^[ref]

A physicist researching high harmonic generation and interactions between lasers and matter.^[ref]